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This article is protected by copyright. All rights reserved.We demonstrate that trimethylamine borane can exhibit desirable piezoelectric and pyroelectric properties. The material was shown to be able operate as a flexible film for both thermal sensing, thermal energy conversion and mechanical sensing with high open circuit voltages (10 V). A piezoelectric coefficient of d33 ≈10-16 pC N-1 , and pyroelectric coefficient of p≈25.8 μC m-2 K-1 were achieved after poling, with high pyroelectric figure of merits for sensing and harvestin
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